福建省先进材料化工基础重点实验室

项生昌教授

个人简介:

项生昌,二级研究员,博士生导师。现任化学与材料学院常务副院长(主持工作)。1993年,1996年本科和硕士毕业于福建师范大学化学系,2003年博士毕业于福州大学化学化工学院。1996年起在福建师范大学任职讲师、副教授、研究员。2003-2007年作为副研究员和博士后加入中科院福建物构所吴新涛院士组,2008-2012年作为研究学者和博士后加入美国Texas大学。2012年回国在福建师范大学工作。长期致力于新型多孔功能材料的设计剪裁、合成新路线和新方法研究,针对能源环境、气候变化、石油化工等工业和应用领域面临的关键科学问题,发展框架构建与功能化,以及孔壁结构优化、孔道功能化和包覆复合等“再功能化”方法,研发高性能多孔材料,推动清洁能源生产、节能减排和环境治理的技术创新。先后主持和承担25项中国国家自然科学基金、973项目、省部级基金和各类人次计划项目的研究,已在国内外期刊上发表130余篇学术论文,含Nature Commun. (3篇), Acc Chem Res (1篇), J. Am. Chem. Soc. (9篇), Angew. Chem. Int. Ed. (4篇)和Energy & Environ Sci(1篇)等,书章3篇,申请发明专利6 件。论文得到了同行的高度评价和大量引用,多篇论文作为研究亮点被Nature Asia- PacificNIST News Letter,《基础科学研究快报》,《中国科学院院刊》等予以报道。Energy & Environ Sci, CrystEngComStruct Bond等期刊邀请撰写相关综述,部分成果获得了国际同行大专家在Nature, Science, Chem Rev, Chem Soc Rev的充分肯定,大幅介绍和正面引用。论文的SCI 引用频次共5000 余次;H-index 指数39。入选教育部新世纪优秀人才支持计划、福建省闽江学者特聘教授,荣获 “创青春”全国大学生“挑战杯”创业计划大赛银奖、2015年中国百篇最具影响力国际学术论文、2014年福建省自然科学优秀学术论文一等奖、ACS 3years Membership Award、UTPA Visiting Scholarship Award等。

研究方向:

  1. 新型孔材料(MOFs, OMMs, PMOs, HOFs, POPs, MIPs)的设计合成、复合与功能化
项生昌教授 科研人员 第2张项生昌教授 科研人员 第3张

Inorg. Chem.2016, 55, 292-299; J. Am. Chem. Soc.2015, 137 (2), 913–918; J. Mater. Chem. A 2015, 3, 593-599;Nature Commun. 2012, 3, 954;Nature Commun.2011, 2, 204; Angew. Chem. Int. Ed.2010, 49, 4615-4618; J. Am. Chem. Soc.2009, 131, 12415-12419;J Am Chem Soc2005, 127, 16352-16353.

  1. 多功能簇合物材料
项生昌教授 科研人员 第4张项生昌教授 科研人员 第5张项生昌教授 科研人员 第6张

Inorg. Chem.2016, 55(1), 292-299; Cryst Growth Deg2015, 15(8), 3847-3852; Chem Commun2014, 50(62), 8558-8560;Inorg Chem2010, 49, 8444-8448;Struct Bond2009, 133, 161-206;J Am Chem Soc2007, 129, 15144-15146; J Am Chem Soc2005, 127, 16352-16353.

  1. 宽温域质子导体材料(in collaboration with Prof. Dr. Zhangjing Zhang)
项生昌教授 科研人员 第7张项生昌教授 科研人员 第8张

Journal of Materials Chemistry A, 2016, 4, DOI:10.1039/C5TA10765B; Inorganic Chemistry, 2016, 55 (2), 983–986; J. Am. Chem. Soc., 2015, 137 (2), 913–918.

  1. 能源气体、重要石化原料的存储和纯化分离
项生昌教授 科研人员 第9张项生昌教授 科研人员 第10张项生昌教授 科研人员 第11张项生昌教授 科研人员 第4张

Chem Eur J, 2016, chem.201505107; Inorg. Chem.2015, ic-2015-023165; Energy Environ. Sci. 2014, 7, 2868-2899 (inside cover);Nature Commun.2012, 3, 954;CrystEngComm2011, 13, 5983-5992;Nature Commun.2011, 2, 204;Angew. Chem. Int. Ed.2010, 49, 4615-4618; J. Am. Chem. Soc.2009, 131, 12415-12419.

  1. 光致变色材料的合成及机理研究(PI: Prof. Dr. Zhangjing Zhang)
  1. MIPs与永久污染物的识别检测和移除(PI: Prof. Dr. Xiuling Ma)

New J. Chem.2016,40, 1649-1654; Monatsh Chem2015,146, 485–491;J. Applied Polymer Sciences, 2014, 131(13), 40491; RSC Adv., 2013, 3, 25396–25402.

团队科研项目:

1、国家自然科学基金,21573042、晶态多孔材料的功能修饰以构建高稳定性、宽温域、高性能质子导体材料、2016/1-2019/12 (PI:张章静)。

2、国家自然科学基金,21273033、室温下碳减排多孔金属有机框架材料的评估、筛选与反馈性设计合成、2013/1-2016/12 (PI:项生昌)。

3、国家自然科学基金,21203024、基于金属-Salen的微孔混金属有机框架对乙炔/乙烯的识别与分离、2013/1-2015/12 (PI:张章静)。

4、国家自然科学基金,21207018、新型溴代阻燃剂分子印迹纳米纤维膜传感器的研制、2013/1-2015/12 (PI:马秀玲)。

5、福建省科技重大项目,2014H6007、低能耗变压吸附脱碳的高端木质活性炭材料的制备与产业化技术研发、2014/11-2017/10 (PI:项生昌)。

6、福建省自然科学基金杰出青年基金,2014J06003、含有裸露金属位点的杂化多孔材料对石化烯炔的识别与分离、2014/1-2016/12 (PI:张章静)。

7、福建省自然科学基金,2015J01039、 TBC分子印迹纳米纤维膜传感器的研制、2015/4-2018/4 (PI:马秀玲)。

8、福建省高校新世纪优秀人才计划,JA13061、多孔有机无机杂化材料、2014/1-2016/12。(PI:张章静)。

9、福建省高校杰出青年科研人才计划,JA12056,基于金属-Salen的微孔混金属有机框架对乙炔/乙烯的识别分离、2014.01-2016.12 (PI:张章静)。

10、福建师范大学首批“宝琛计划”科技创新团队,IRTL1202、面向能源环境关键问题的孔材料设计、2013/1-2017/12 (PI:项生昌)。

11、结构化学国家重点实验室科学基金,20130004、微孔混金属有机框架对乙炔/乙烯的识别与分离、2013.01-2015.12 (PI:张章静)。

12、结构化学国家重点实验室科学基金,20150024、沼气脱碳用的多孔MOF-GO 复合材料的结构调控与性能研究、2015/01-2017/12 (PI:项生昌)。

13、福建省自然科学基金,23161072、含开放功能位点的MOFs的设计合成及其在乙炔混合物分离中的应用、2016/04-2019/04 (PI:王丽华)。

Publications:

2016






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43.

Yingxiang Ye,+ Xiuzhen Wu, + Zizhu Yao, Ling Wu, Zetao Cai, Lihua Wang, Xiuling Ma, Qian-Huo Chen, Zhangjing Zhang,* and Shengchang Xiang,* Metal-Organic Frameworks with Large Breathing Effect to Host Hydroxyl Compounds for High Anhydrous Proton Conductivity over a Wide Temperature Range from Subzero to 125 oC, Journal of Materials Chemistry A, 2016, 4, 4062 – 4070, DOI: 10.1039/C5TA10765B


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42.

Zizhu Yao, Zhangjing Zhang, Lizhen Liu, Ziyin Li, Wei Zhou, Yunfeng Zhao, Yu Han, Banglin Chen, Rajamani Krishna and Shengchang Xiang,* Extraordinary Separation Performance towards Acetylene Containing Mixtures on Microporous MOFs with Open O Donor Sites and Tunable Robustness via Control of Helical Chains SBUs, Chemistry-A European Journal, 2016, chem.201505107



41.

Xuelian Su, Zizhu Yao, Yingxiang Ye, Heng Zeng, Gang Xu, Ling Wu, Xiuling Ma, Qian-Huo Chen, Lihua Wang, Zhangjing Zhang* and Shengchang Xiang,* Forty-fold Enhanced Intrinsic Proton Conductivity in Coordination Polymers with Same Proton-Conducting Pathway by Tuning Metal Cation Nodes Inorganic Chemistry, 2016, 55 (2), 983–986 DOI: 10.1021/acs.inorgchem.5b02686


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40.


Yingxiang Ye, Shunshun Xiong, Xiaonan Wu, Liuqin Zhang,Ziyin Li, Lihua Wang,* Xiuling Ma, Qian-Huo Chen, Zhangjing Zhang, and Shengchang Xiang,*Microporous Metal-Organic Framework Stabilized by Balanced Multiple Host-Couteranion Hydrogen Bonding Interactions for High- density CO2 Capture at Ambient ConditionsInorganic Chemistry,2016, 55(1), 292-299 DOI:

10.1021/acs.inorgchem.5b02316



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39.

Xiuling Ma, Jiaxiang Liu, Dan Wu, Zhangjing Zhang, Lihua Wang,* Qian-Huo Chen, and Shengchang Xiang,* Ultrasensitive Sensing Tris(2,3-dibromopropyl) Isocyanurate Based on the Synergistic Effect of Amino and Hydroxyl Groups of Molecularly Imprinted Poly (o-aminophenol) Film,New Journal of Chemistry2016, 40, 1649-1654. DOI: 10.1039/C5NJ02031J


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38.

Lizhen Liu,Yingxiang Ye, Zizhu Yao,Liuqin Zhang, Ziyin Li, Lihua Wang*, Xiuling Ma, Qian-Huo Chen, Zhangjing Zhang, and Shengchang Xiang* A Hierarchically Porous Metal- Organic Framework from Semirigid Ligand for Gas AdsorptionChinese Journal of Chemistry2016,34,215-219 DOI:/10.1002/cjoc.201500617

2015


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37.


Yuan Chen, Ziyin Li, Qing Liu, Yangcan Shen, Xiuzhen Wu, Dandan Xu, Xiuling Ma, Lihua Wang, Qian-Huo Chen, Zhangjing Zhang,* Shengchang Xiang,* Microporous Metal- Organic Framework with Lantern-like Dodecanuclear Metal Coordination Cages as Nodes for Selective Adsorption of C2/C-1 Mixtures and Sensing of Nitrobenzene,Crystal Growth & Design, 2015, 15(8): 3847-3852.

DOI: 10.1021/acs.cgd.5b00473


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36.

Ganggang Chang, Bin Li, Hailong Wang, Zongbi Bao, Taner Yildirim, Zizhu Yao, Shengchang Xiang, Wei Zhou, Banglin Chen,* A microporous metal-organic framework with polarized trifluoromethyl groups for high methane storage,Chemical Communications, 2015, 51(79): 14789- 14792. DOI: 10.1039/c5cc05850c



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35.


Xing Duan, Chuande Wu, Shengchang Xiang, Wei Zhou, Taner Yildirim, Yuanjing Cui, Yu Yang, Banglin Chen,* Guodong Qian,* Novel Microporous Metal-Organic Framework Exhibiting High Acetylene and Methane Storage Capacities,Inorganic Chemistry, 2015, 54(9): 4377-4381.

DOI: 10.1021/acs.inorgchem.5b00194


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34.

Tong-Liang Hu, Hailong Wang, Bin Li, Rajamani Krishna, Hui Wu, Wei Zhou, Yunfeng Zhao, Yu Han, Xue Wang, Weidong Zhu, Zizhu Yao, Shengchang Xiang, Banglin Chen,*Microporous metal-organic framework with dual functionalities for highly efficient removal of acetylene from ethylene/acetylene mixtures. Nature Communications, 2015, 6:7382. DOI: 10.1038/ncomms8328



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33.

Hailong Wang, Bin Li, Hui Wu, Tong-Liang Hu, Zizhu Yao, Wei Zhou,* Shengchang Xiang, Banglin Chen,*A Flexible Microporous Hydrogen-Bonded Organic Framework for Gas Sorption and Separation, Journal of the American Chemical Society, 2015, 137(31): 9963-9970


DOI: 10.1021/jacs.5b05644


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32.


Lihua Wang,* Yingxiang Ye, Liuqin Zhang, Qianhuo Chen, Xiuling Ma, Zhangjing Zhang, Shengchang Xiang,*A 3D- diamond-like metal-organic framework: Crystal structure, nonlinear optical effect and high thermal stability, Inorganic Chemistry Communications, 2015, 60:19-22

DOI: 10.1016/j.inoche.2015.07.015



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31.


Hui-Jie Lun, Sa-Sa Cui, Hai-Jiao Li, Qi Ping, Hao-Han Song, Ya-Min Li,* Yu Ru, Yan-Long Bai, Shengchang Xiang,* A chiral coordination polymer with double coaxially nested helical chains exhibiting spin-canting antiferromagnetism, CrystEngComm2015, 17(37): 7029-7033,

DOI: 10.1039/c5ce01378j.


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30.

Yingxiang Ye, Liuqin Zhang, Qinfang Peng, Guan-E Wang, Yangcan Shen, Ziyin Li, Lihua Wang, Xiuling Ma, Qian-Huo Chen, Zhangjing Zhang,* Shengchang Xiang,* High Anhydrous Proton Conductivity of Imidazole-Loaded Mesoporous Polyimides over a Wide Range from Subzero to Moderate Temperature, Journal of the American Chemical Society,2015, 137(2), 913–918



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29.

Yangcan Shen, Ziyin Li, Lihua Wang, Yingxiang Ye, Qing Liu, Xiuling Ma, Qianhuo Chen, Zhangjing Zhang* and Shengchang Xiang,* Armored Cobalt-Citrate Framework with Graphene Oxide Exhibiting Improved Thermal Stability and Selectivity for Biogas Decarburization, Journal of Materials Chemistry A, 2015, 3 (2), 593 – 599. DOI: 10.1039/C4TA04770B



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28.

Xiuling Ma, Dan Wu, Limei Huang, Zhenyue Wu, Shengchang Xiang, Sheng Chen,* Sensing 2,4,6-tribromophenol based on molecularly imprinted technology, Monatsh Chem, 2015, 146:485–491

2014


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27.

Hussah Alawisi, Bin Li,* Khalid Alfooty, Ling Wu, Shengchang Xiang, Hailong Wang, Banglin Chen,*A two dimensional microporous metal-organic framework for selective gas separation, Inorganic Chemistry Communications, 2014, 50:106-109. DOI: 10.1016/j.inoche.2014.10.023


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26.


Zhangjing Zhang, Zi-Zhu Yao, Shengchang Xiang,* Banglin Chen,* Perspective of microporous metal-organic frameworks for CO2 capture and separation, Energy &

Environmental Science2014, 7(9): 2868-2899, DOI: 10.1039/c4ee00143e



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25.

Ya-Min Li, Hui-Jie Lun, Chang-Yu Xiao, Yan-Qing Xu, Ling Wu, Jing-He Yang, Jing-Yang Niu, Sheng-Chang Xiang,* A bilayer triangular lattice with crown-like Co-7 spin cluster SBUs exhibiting high spin frustration, Chemical Communications, 2014, 50(62): 8558-8560, DOI: 10.1039/c4cc02910k


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24.

Peng Li, Yabing He, Jie Guang, Linghong Weng, John Cong- Gui Zhao, Shengchang Xiang, Banglin Chen,* A Homochiral Microporous Hydrogen-Bonded Organic Framework for Highly Enantioselective Separation of Secondary Alcohols, Journal of the American Chemical Society2014, 136(2): 547-549, DOI: 10.1021/ja4129795


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23.


Xiu-Li Yang, Chao Zou, Yabing He, Min Zhao, Banglin Chen,* Shengchang Xiang, Michael O'Keeffe, Chuan-De Wu,* A Stable Microporous Mixed-Metal Metal-Organic Framework with Highly Active Cu2+ Sites for Efficient Cross- Dehydrogenative Coupling Reactions, Chemistry-A European Journal, 2014, 20(5): 1447-1452, DOI: 10.1002/chem.201303615


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22.

Wei-Chen Lin, Wei-Gang Guo, Li-Hua Wang, Xiu-Ling Ma, Zhang-Jing Zhang,* Sheng-Chang Xiang, Synthesis, Structure and Characterization of a new Zinc Citrate Complex Containing Ladder-like Chains, Chinese Journal of Structural Chemistry, 2014,33(4) 591-596.



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21.


Xiuling Ma, Zhangjing Zhang, Ying Zheng, Zhen Chen, Shengchang Xiang,* Water-compatible Imprinted Polymers Based on CS@SiO2 Particles for Selective Recognition of Naringin, Journal of Applied Polymer Sciences,

2014,131(13), 40491

2013


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20.

Xiuling Ma,* Jiaxiang Liu, Zhangjing Zhang, Lihua Wang, Zhen Chen, Shengchang Xiang,* The cooperative utilization of imprinting, electro-spinning and a pore-forming agent to synthesize b-cyclodextrin polymers with enhanced recognition of naringin, RSC Advances2013, 3, 25396–25402



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19.

Xu Hui, He Yabing, Zhang Zhangjing, Shengchang Xiang, Jianfeng Cai, Yuanjing Cui, Yu Yang, Guodong Qian,* Banglin Chen,* A cationic microporous metal-organic framework for highly selective separation of small hydrocarbons at room temperature, Journal of Materials Chemistry A2013, 1(34), 9916-9921



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18.

Yabing He,* Shengchang Xiang, Zhangjing Zhang, Shunshun Xiong, Chuande Wu, Wei Zhou, Taner Yildirim, Rajamani Krishna, Banglin Chen,* A microporous metal-organic framework assembled from an aromatic tetracarboxylate for H2 purification, Journal of Materials Chemistry A2013, 1(7), 2543-2551


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17.


Xing Duan, Jiancan Yu, Jianfeng Cai, Yabing He, Chuande Wu, Wei Zhou, Taner Yildirim, Zhangjing Zhang, Shengchang Xiang, Michael O'Keeffe, Banglin Chen,* Guodong Qian,* A microporous metal-organic framework of a rare sty topology

for high CH4 storage at room temperature, Chemical Communications2013, 49(20), 2043-2045


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16.


Hui Xu, Jianfeng Cai, Shengchang Xiang, Zhangjing Zhang, Chuande Wu, Xiangtang Rao, Yuanjing Cui, Yu Yang, Rajamani Krishna, Banglin Chen,* Guodong Qian,* A microporous metal-organic framework with both open metal and Lewis basic pyridyl sites for highly selective C2H2/CH4 and

C2H2/CO2 gas separation at room temperature, Journal of Materials Chemistry A2013, 1(1), 77-81.



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15.


Guohui Chen, Zhangjing Zhang, Shengchang Xiang, Banglin Chen,* A microporous metal-organic framework with Lewis basic pyridyl sites for selective gas separation of

C2H2/CH4 and CO2/CH4 at room temperature,


CrystEngComm2013, 15(26), 5232-5235


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14.

Sridhar Regati, Yabing He, Muralidhara Thimmaiah, Peng Li, Shengchang Xiang, Banglin Chen,* Cong-Gui John Zhao,* Enantioselective ring-opening of meso-epoxides by aromatic amines catalyzed by a homochiral metal-organic framework, Chemical Communications2013, 49(84), 9836-9838


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13.

Yabing He,* Zhiyong Guo, Shengchang Xiang, Zhangjing Zhang, Wei Zhou, Frank R. Fronczek, Sean Parkin, Stephen T. Hyde, Michael O'Keeffe, Banglin Chen,* Metastable Interwoven Mesoporous Metal-Organic Frameworks,


Inorganic Chemistry2013, 52(19), 11580-11584



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12.


Rebecca A. Joy, Hadi Arman, Shengchang Xiang, et al. Synthesis, crystal structure, magnetic and electrochemical studies of two copper complexes with carboxylate rich dinucleating ligand,Inorganic Chimica Acta2013, 394, 220-

228

2012



11.

Shengchang Xiang, Yabing He, Zhangjing Zhang, Hui Wu, Wei Zhou, Rajamani Krishna, Banglin Chen,* Microporous metal-organic framework with potential for carbon dioxide capture at ambient conditions, Nature Communications, 2012, 3, 954.


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10.

Lei Shen, Shuo-Wang Yang,* Shengchang Xiang, Tao Liu, Bangchuan Zhao, Man-Fai Ng, Jörg Göettlicher, Jiabao Yi, Sean Li, Lan Wang, Jun Ding, Banglin Chen, Su-Huai Wei, Yuan Ping Feng,* Origin of long-range ferromagnetic ordering in metal-organic frameworks with antiferromagnetic dimeric-Cu(II) building units, Journal of the American Chemical Society, 2012, 134 , 17286–17290



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9.

Madhab C. Das, Qunsheng Guo, Yabing He, Jaheon Kim, Cong-Gui Zhao, Kunlun Hong, Shengchang Xiang, Zhangjing Zhang, K. Mark Thomas, Rajamani Krishna, and Banglin Chen, Interplay of metalloligand and organic ligand to tune micropores within isostructural mixed-metal organic frameworks (M'MOFs) for their highly selective separation of chiral and achiral small molecules, Journal of the American Chemical Society, 2012, 134(20), 8703-8710.


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8.

Yabing He, Shengchang Xiang, Zhangjing Zhang, Shunshun Xiong, Frank R. Fronczek, Rajamani Krishna, Michael O'Keeffe and Banglin Chen,* A microporous lanthanide-tricarboxylate framework with the potential for purification of natural gas, Chemical Communications, 2012, 48, 10856-10858


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7.

Qilong Zhu, Shengchang Xiang, Tianlu Sheng, Daqiang Yuan, Chaojun Shen, Chunhong Tan, Shengmin Hu and Xintao Wu,* A series of goblet-like heterometallic pentanuclear [Ln(III)Cu(4)(II)] clusters featuring ferromagnetic coupling and single-molecule magnet behavior, Chemical Communications, 2012, 48, 10736-10738



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6.

Yabing He, Zhangjing Zhang, Shengchang Xiang, Frank R. Fronczek, Rajamani Krishna and Banglin Chen,* A robust doubly interpenetrated metal-organic framework constructed from a novel aromatic tricarboxylate for highly selective separation of small hydrocarbons, Chemical Communications, 2012, 48, 6493-6495



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5.

Yabing He, Zhangjing Zhang, Shengchang Xiang, Hui Wu, Frank R. Fronczek, Wei Zhou, Rajamani Krishna, Michael O'Keeffe, Banglin Chen,* High separation capacity and selectivity of C2 hydrocarbons over methane within a microporous metal-organic framework at room temperature, Chemistry – a European Journal,2012, 18, 1901-1904


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4.

Yabing He, Zhangjing Zhang, Shengchang Xiang, Frank R. Fronczek, Rajamani Krishna, Banglin Chen,* A microporous metal-organic framework for highly selective separation of acetylene, ethylene, and ethane from methane at room temperature, Chemistry – a European Journal, 2012, 18, 613-619.



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3.

Yun-Xia Hu, Hai-Bo Ma, Bo Zheng, Wen-Wei Zhang,* Shengchang Xiang, Lu Zhai, Li-Feng Wang, Banglin Chen, Xiao-Ming Ren, and Junfeng Bai,* Three Novel Isomeric Zinc Metal-Organic Frameworks from a Tetracarboxylate Linker, Inorganic Chemistry, 2012, 51, 7066-7074



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2.

Jianshan Chen, Tianlu Sheng, Shengmin Hu, Shengchang Xiang, Ruibiao Fu, Qilong Zhu, Xintao Wu,* Homochiral coordination polymers constructed from aminocarboxylate derivates: Effect of bipyridine on the amidation reaction, Journal of Solid State Chemistry,2012,192, 255-262


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1.

Zhangjing Zhang, Shengchang Xiang,* Kunlun Hong, Madhab, C. Das, Hadi D. Arman, Maya Garcia, Jalal U. Mondal, K. Mark Thomas, and Banglin Chen,* Triple Framework Interpenetration and Immobilization of Open Metal Sites within a Microporous Mixed Metal-Organic Framework for Highly Selective Gas Adsorption, Inorganic Chemistry, 2012, 51, 4947-4953

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